Impact of Sulfur Dioxide on the Terrestrial Carbon Cycle

Abstract

This paper updates the results obtained earlier with the climate model developed at the A.M. Obukhov Institute of Atmospheric Physics of the Russian Academy of Sciences (IAP RAS CM) and describing the impact of atmospheric sulfur dioxide on the terrestrial carbon cycle. Since no global data are available for the near-surface SO₂ concentration, a statistical model was used to reconstruct its concentration from appropriate data on surface sulfate concentrations; the coefficients of this model were tuned by using the output of the RAMS-CMAQ atmospheric chemistry and transport model. The results obtained in this study are generally consistent with data reported earlier. Specifically, the most significant SO₂ impact on the terrestrial carbon cycle was found to be for southeastern North America and for Europe. However, this impact for southeastern Asia obtained in this study is considerably weaker than the value obtained earlier, which can be explained by the excessive moisture content in the atmosphere used in the IAP RAS CM for this region.