Sorption of Radionuclides from the Primary Circuits of Reactors with Pb–Bi Coolant onto the Surface of Structural Materials of the Reactor Core

Abstract

Sorption and phase distribution of ⁵⁴Mn, ⁵⁹Fe, ⁶⁰Со, ¹⁰⁶Ru, ¹²⁵Sb, ¹³⁷Cs, ¹⁴⁴Се, ^154,155Eu, and ^235,238U radionuclides in contact of the Pb–Bi melt with the steel surface were studied. Radionuclides of the elements with the minimal oxygen affinity (Ru, Te, and Sb) remain mainly in the coolant melt and are weakly sorbed onto the solid phase. The other fission product radionuclides having higher oxygen affinity are sorbed onto the surface of steel structural materials. The sorption increases at 350–400°С.