The Gd–Ce Cross-Relaxation Effects in ODMR via Ce3+ Emission in Garnet Crystals


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Electron paramagnetic resonance (EPR) in the ground state of Gd3+ ions in (LuGd)3 Al5O12 single crystals has been found by monitoring the Ce3+ photoluminescence intensity under circularly polarized excitation in the presence of the 35 GHz microwave field. Due to spin selection rules for optical transitions, the circularly polarized excitation allowed monitoring the populations of the Ce3+ ground-state spin sublevels, which can be changed at the EPR of Gd3+ due to Gd–Ce cross relaxation.

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N. Romanov

Ioffe Institute

编辑信件的主要联系方式.
Email: nikolai.romanov@mail.ioffe.ru
俄罗斯联邦, 26 Politekhnicheskaya, St Petersburg, 194021

D. Tolmachev

Ioffe Institute

Email: nikolai.romanov@mail.ioffe.ru
俄罗斯联邦, 26 Politekhnicheskaya, St Petersburg, 194021

A. Gurin

Ioffe Institute

Email: nikolai.romanov@mail.ioffe.ru
俄罗斯联邦, 26 Politekhnicheskaya, St Petersburg, 194021

Yu. Uspenskaya

Ioffe Institute

Email: nikolai.romanov@mail.ioffe.ru
俄罗斯联邦, 26 Politekhnicheskaya, St Petersburg, 194021

E. Edinach

Ioffe Institute

Email: nikolai.romanov@mail.ioffe.ru
俄罗斯联邦, 26 Politekhnicheskaya, St Petersburg, 194021

H. Asatryan

Ioffe Institute

Email: nikolai.romanov@mail.ioffe.ru
俄罗斯联邦, 26 Politekhnicheskaya, St Petersburg, 194021

A. Badalyan

Ioffe Institute

Email: nikolai.romanov@mail.ioffe.ru
俄罗斯联邦, 26 Politekhnicheskaya, St Petersburg, 194021

P. Baranov

Ioffe Institute

Email: nikolai.romanov@mail.ioffe.ru
俄罗斯联邦, 26 Politekhnicheskaya, St Petersburg, 194021

A. Petrosyan

Institute for Physical Research, NAS RA

Email: nikolai.romanov@mail.ioffe.ru
亚美尼亚, Ashtarak-2, Yerevan, 0203

H. Wieczorek

Philips Research

Email: nikolai.romanov@mail.ioffe.ru
荷兰, High Tech Campus 34, AE Eindhoven, 5656

C. Ronda

Philips Research

Email: nikolai.romanov@mail.ioffe.ru
荷兰, High Tech Campus 34, AE Eindhoven, 5656


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