


卷 104, 编号 8 (2016)
- 年: 2016
- 文章: 12
- URL: https://journals.rcsi.science/0021-3640/issue/view/9698
Condensed Matter
Simulated Cu–Zr glassy alloys: the impact of composition on icosahedral order
摘要
The structural properties of the simulated CuαZr1-α glassy alloys are studied in the wide range of the copper concentration to clarify the impact of the composition on the number density of the icosahedral clusters. Both bond orientational order parameters and Voronoi tessellation methods are used to identify these clusters. Our analysis shows that abundance of the icosahedral clusters and the chemical composition of these clusters are essentially nonmonotonic versus and demonstrate local extrema. That qualitatively explains the existence of pinpoint compositions of high glass-forming ability observing in Cu Zr alloys. Finally, it has been shown that Voronoi method overestimates drastically the abundance of the icosahedral clusters in comparison with the bond orientational order parameters one.



Ab initio study of magnetic properties in the adsorption of transition-metal atoms on arsenene
摘要
The magnetic properties of adsorption of different transition-metal (TM) atoms (Co, Cu, Mn, Fe, and Ni) on arsenene are investigated using density functional theory (DFT). Magnetism appears in the cases of Co, Mn, and Fe. Among all the magnetic cases, the TM atom prefers the same adsorption site. Then, we further study the interaction in two-TM-adsorbed system and different magnetic states are observed. Our results show that both nonmagnetic and ferromagnetic states exist in two-Co-adsorbed system and the p-d hybridization mechanism results in its ferromagnetic state. However, for two Mn and two Fe adsorbed systems, an AFM interaction is found, which could be reasonably explained by the superexchange mechanism. Such multiple magnetic properties may suggest promising applications of TM-adsorbed arsenene in the future.



Coherent cluster atomic ordering in the Fe-27Al intermetallic compound
摘要
Neutron diffraction studies of the Fe0.735Al0.265 compound are performed in a wide temperature range (20–900°C) in order to determine its structural states and the mechanism of ordering of atoms. The combination of high-resolution diffraction and the real-time detection of diffraction spectra makes it possible to establish that, in contrast to traditional notions, the structure of this compound at room temperature is a phase with only a partially ordered arrangement of Fe and Al in a unit cell. A completely ordered phase (such as Fe3Al) is present in the form of mesoscopic (~200Å) clusters coherently incorporated into the disordered matrix of the main phase. After the transition of the sample to a disordered state (T> 740°С) and slow cooling to room temperature, the size of structurally ordered clusters increases to ~900 Å. A high contrast in the coherent neutron scattering lengths of iron and gallium nuclei allows the accurate determination of the temperature dependence of the occupancy factors of sites by Fe and Al atoms up to a phase transition to the disordered state.



Boson peak in various random-matrix models
摘要
A so-called boson peak in the reduced density g(ω)ω2 of vibrational states is one of the most universal properties of amorphous solids (glasses). It quantifies the excess density of states above the Debye value at low frequencies ω. Its nature is not fully understood and, at a first sight, is nonuniversal. It is shown in this work that, under rather general assumptions, the boson peak emerges in a natural way in very dissimilar models of stable random dynamic matrices possessing translational symmetry. This peak can be shifted toward both higher and lower frequencies (down to zero frequency) by varying the parameters of the distribution and the degree of disorder in the system. The frequency ωb of the boson peak appears to be proportional to the elastic modulus E of the system in all cases under investigation.



Spatial–frequency selection of magnetostatic waves in a two-dimensional magnonic crystal lattice
摘要
Features of the propagation of magnetostatic waves in a tangentially magnetized magnonic crystal structure based on iron–yttrium garnet with a two-dimensional array of grooves on the surface are studied. Numerical simulation is performed by the finite element method and the dispersion characteristics and the spatial distribution of fields of eigenmodes of surface magnetostatic waves propagating in this structure are calculated. The characteristics of waves in the magnonic crystal structure are experimentally studied by means of Brillouin scattering. It is shown that the formation of waveguide channels is possible when the frequency of the input signal is close to the frequency of the band gap of the structure.



Multiferroic based on metal–organic dimers with the Dzyaloshinskii–Moriya effect
摘要
A magnetoelectric effect has been found at room temperature in a polymer composite—polystyrene–metal–organic manganese dimers with ligands of spatially hindered phenol. It is shown that these metal-organic manganese dimers implement the Dzyaloshinskii–Moriya interaction and are weakly ferromagnetic. It is suggested that a new class of high-temperature multiferroics can be created on the basis of such molecular structures.



Fields, Particles, and Nuclei
Polarization effects of the τ → K–π0ντ process in the Nambu–Jona-Lasinio model
摘要
The polarization effects of the τ → K–π0ντ process are described in the framework of the Nambu–Jona-Lasinio model. The intermediate vector meson K*(892) is taken into account. The contribution of these effects to the differential decay width is obtained.



Proton halo in the 13N nucleus
摘要
We demonstrate that the radii of excited nuclear states can be estimated using the (3He, t) charge-exchange reaction and relying on the modified diffraction model. The radius of the N excited state with an excitation energy of E*=2.73 MeV, which lies in a continuous spectrum, is determined. The radius of this state proves to be close to that of the mirror 3.09-MeV state of the 13С nucleus, which possesses a neutron halo but lies in a discrete spectrum. Thereby, we demonstrate that the 2.37-MeV state of the 13N nucleus has a proton halo. The analysis is based on published measurements of differential cross sections for relevant reactions.



Miscellaneous
Thermal melting and ablation dynamics on a femtosecond laser-heated highly-oriented pyrolytic graphite surface
摘要
Time-resolved optical reflection microscopy studies demonstrate spatiotemporal dynamics of melting and ablation of graphite surface molten by single IR femtosecond laser pulses, which are revealed by monitoring picosecond oscillations of the probe reflectivity modulated by transient acoustic reverberations in the surface melt. Temporal periods and amplitudes of the reverberations are affected through transient variations of melt thickness and acoustic impedance by melting, thermal expansion, spallation and fragmentation processes, thus enabling quantitative evaluation of their contributions and basic parameters.



Plasma, Hydro- and Gas Dynamics
Enhancement of waves at rotational oscillations of a liquid
摘要
Flows of a viscous incompressible fluid in a spherical layer that are due to rotational oscillations of its inner boundary at two frequencies with respect to the state of rest are numerically studied. It is found that an increase in the amplitude of oscillations of the boundary at the higher frequency can result in a significant enhancement of the low-frequency mode in a flow near the outer boundary. The direction of propagation of the low-frequency wave changes from radial to meridional, whereas the high-frequency wave propagates in the radial direction in a limited inner region of the spherical layer. The role of the meridional circulation in the energy exchange between spaced waves is demonstrated.



Scientific Summaries
Theory of coherent charge transport in junctions involving unconventional superconducting materials
摘要
Recent theoretical studies of coherent charge transport in junctions involving unconventional superconducting materials such as high-temperature superconducting iron-based pnictides (FeBS) and in structures with induced superconductivity which are formed of a thin metal layer with spin–orbit coupling in contact with an s-wave superconductor (SSO) are reported. The theoretical analysis is performed with our unified approach based on the tight-binding method and boundary conditions obtained for it. This approach makes it possible to take into account a complex nonparabolic and anisotropic spectrum of normal excitations in unconventional superconducting materials and their multiband character, as well as unusual types of symmetries of the superconducting order parameter in them. The possibility of a semiclassical description in the case of intraorbital superconducting pairing is demonstrated. The method of calculations and their results are presented for the conductivities of junctions between a normal metal and unconventional superconducting materials, as well as for the Josephson current. Comparison with the experiment for the junction with FeBS is performed and indicates the presence of the unusual s± symmetry of the order parameter. An experiment is proposed to test our theoretical results for SSO.



Anomalies of the electronic structure and physical properties of rare-earth cobaltites near spin crossover
摘要
The features of the characteristics of LnCoO3 cobaltites, where Ln is a rare-earth element, are discussed. Both experiment and theory demonstrate that their essentials are related to the low-spin ground state of cobalt ions. The thermally induced occupation of the excited high-spin state gives rise to peaks in the magnetic susceptibility, specific heat, and thermal expansion, as well as to a smooth insulator–metal transition. The analysis is based both on the data from the current literature concerning LaCoO3 and in many aspects on our own studies of GdCoO3 and La1−xGdxCoO3 solid solutions.


