Radionuclides Distribution and its Sorption Behavior in the Surface Layer of the Kara Sea Bottom Sediments


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Abstract

Abstract—The sorption characteristics of the Kara sea bottom sediments were investigated. The sediments were collected during scientific expedition of the R/V Akademik Mstislav Keldysh (Cruise AMK-66). The mineral and fraction composition of the sediments was determined. It has been found that 137Cs is sorbed mainly by an ion exchange mechanism because of the clay minerals presence in sediments. At the same time, 243Am and 90Sr sorbed from seawater by the surface complexation mechanism. It has been established that the sorption kinetics of 243Am, 137Cs, and 90Sr is about 20 hours, 2 hours, and less than an hour, respectively. The Cs and Am sorption isotherms in experiments with sea and deionized water are described by the Henry equation. The Sr behavior in the deionized and sea water is described by the Langmuir and Freindlikh equations, respectively.

About the authors

N. V. Kuzmenkova

Vernadsky Geochemistry Institute RAS; Lomonosov Moscow State University, Chemistry department

Author for correspondence.
Email: kouzmenkova@mail.ru
Russian Federation, Kosygina str. 19, Moscow, 119991; Leninskye g. 1, Moscow, 119991

V. V. Krupskaya

Geology of Ore Deposits Institute RAS

Email: kouzmenkova@mail.ru
Russian Federation, Staromonetny per. 35, Moscow, 119017

E. V. Duriagina

Lomonosov Moscow State University, Chemistry department

Email: kouzmenkova@mail.ru
Russian Federation, Leninskye g. 1, Moscow, 119991

I. N. Semenkov

Lomonosov Moscow State University, Geography department

Email: kouzmenkova@mail.ru
Russian Federation, Leninskye g. 1, Moscow, 119991

S. E. Vinokurov

Vernadsky Geochemistry Institute RAS

Email: kouzmenkova@mail.ru
Russian Federation, Kosygina str. 19, Moscow, 119991

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