Cascade χ(3)-Nonlinear Processes in a New SRS-Active Ca2MgSi2O7 Crystal


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Stimulated Raman scattering in magnesium silicate Ca2MgSi2O7, which enters the family of \(D_{{2d}}^{3}\)‑tetragonal acentric crystals with a melilite structure, has been observed. The recorded components of Stokes and anti-Stokes χ(3)-nonlinear lasing are identified with two SRS-active modes, ωSRS1 ~ 908 cm–1 and ωSRS2 ~ 668 cm–1, which also manifest themselves in the generation of combined phonon modes ωSRS3C ~ 170 cm–1 and ωSRS4C ~ 1270 cm–1.

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A. Kaminskii

Shubnikov Institute of Crystallography, Federal Scientific Research Center Crystallography and Photonics, Russian Academy of Sciences

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Email: kaminalex@mail.ru
俄罗斯联邦, Moscow, 119333

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